Description

Signatures of nonlinear and non-Gaussian dynamics in time-resolved linear and nonlinear (correlation) 2D spectra are analyzed in a model considering a linear plus quadratic dependence of the spectroscopic transition frequency

Signatures of nonlinear and non-Gaussian dynamics in time-resolved linear and nonlinear (correlation) 2D spectra are analyzed in a model considering a linear plus quadratic dependence of the spectroscopic transition frequency on a Gaussian nuclear coordinate of the thermal bath (quadratic coupling). This new model is contrasted to the commonly assumed linear dependence of the transition frequency on the medium nuclear coordinates (linear coupling).

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Date Created
  • 2014-07-17
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  • Text
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    Identifier
    • Digital object identifier: 10.1021/jp500733s
    • Identifier Type
      International standard serial number
      Identifier Value
      1520-6106
    • Identifier Type
      International standard serial number
      Identifier Value
      1520-5207
    Note
    • This document is the Accepted Manuscript version of a Published Work that appeared in final form in JOURNAL OF PHYSICAL CHEMISTRY B, copyright American Chemical Society after peer review and technical editing by the publisher. To access the final published work, see http://dx.doi.org/10.1021/jp500733s, opens in a new window

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    This is a suggested citation. Consult the appropriate style guide for specific citation guidelines.

    Dinpajooh, Mohammadhasan, & Matyushov, Dmitry V. (2014). Non-Gaussian Lineshapes and Dynamics of Time-Resolved Linear and Nonlinear (Correlation) Spectra. JOURNAL OF PHYSICAL CHEMISTRY B, 118(28), 7925-7936. http://dx.doi.org/10.1021/jp500733s

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