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Description
Among volcanic gases, sulfur dioxide (SO2) is by far the most commonly measured. More than a monitoring proxy for volcanic degassing, SO2 has the potential to alter climate patterns. Persistently active explosive volcanoes are characterized by short explosive bursts, which often occur at periodic intervals numerous times per day,

Among volcanic gases, sulfur dioxide (SO2) is by far the most commonly measured. More than a monitoring proxy for volcanic degassing, SO2 has the potential to alter climate patterns. Persistently active explosive volcanoes are characterized by short explosive bursts, which often occur at periodic intervals numerous times per day, spanning years to decades. SO2 emissions at those volcanoes are poorly constrained, in large part because the current satellite monitoring techniques are unable to detect or quantify plumes of low concentration in the troposphere. Eruption plumes also often show high concentrations of ash and/or aerosols, which further inhibit the detection methods. In this work I focus on quantifying volcanic gas emissions at persistently active explosive volcanoes and their variations over short timescales (minutes to hours), in order to document their contribution to natural SO2 flux as well as investigate the physical processes that control their behavior.

In order to make these measurements, I first develop and assemble a UV ground-based instrument, and validate it against an independently measured source of SO2 at a coal-burning power plant in Arizona. I establish a measurement protocol and demonstrate that the instrument measures SO2 fluxes with < 20 % error. Using the same protocol, I establish a record of the degassing patterns at Semeru volcano (Indonesia), a volcano that has been producing cycles of repeated explosions with periods of minutes to hours for the past several decades. Semeru produces an average of 21-71 tons of SO2 per day, amounting to a yearly output of 8-26 Mt.

Using the Semeru data, along with a 1-D transient numerical model of magma ascent, I test the validity of a model in which a viscous plug at the top of the conduit produces cycles of eruption and gas release. I find that it can be a valid hypothesis to explain the observed patterns of degassing at Semeru. Periodic behavior in such a system occurs for a very narrow range of conditions, for which the mass balance between magma flux and open-system gas escape repeatedly generates a viscous plug, pressurizes the magma beneath the plug, and then explosively disrupts it.
ContributorsSmekens, Jean-François (Author) / Clarke, Amanda (Thesis advisor) / Christensen, Philip R. (Philip Russel) (Committee member) / Williams, Stanley (Committee member) / Burton, Michael (Committee member) / Fink, Jonathan (Committee member) / Moore, Gordon (Committee member) / Arizona State University (Publisher)
Created2015
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Description
Assessments for the threats posed by volcanic eruptions rely in large part on the accurate prediction of volcanic plume motion over time. That predictive capacity is currently hindered by a limited understanding of volcanic plume dynamics. While eruption rate is considered a dominant control on volcanic plume dynamics, the effects

Assessments for the threats posed by volcanic eruptions rely in large part on the accurate prediction of volcanic plume motion over time. That predictive capacity is currently hindered by a limited understanding of volcanic plume dynamics. While eruption rate is considered a dominant control on volcanic plume dynamics, the effects of variable eruption rates on plume rise and evolution are not well understood. To address this aspect of plume dynamics, I conducted an experimental investigation wherein I quantified the relationship between laboratory jet development and highly-variable discharge rates under conditions analogous to those which may prevail in unsteady, short-lived explosive eruptions. I created turbulent jets in the laboratory by releasing pressurized water into a tank of still water. I then measured the resultant jet growth over time using simple video images and particle image velocimetry (PIV). I investigated jet behavior over a range of jet Reynolds numbers which overlaps with estimates of Reynolds numbers for short-duration volcanic plumes. By analysis of the jet boundary and velocity field evolution, I discovered a direct relationship between changes in vent conditions and jet evolution. Jet behavior evolved through a sequence of three stages - jet-like, transitional, and puff-like - that correlate with three main injection phases - acceleration, deceleration and off. While the source was off, jets were characterized by relatively constant internal velocity distributions and flow propagation followed that of a classical puff. However, while the source was on, the flow properties - both in the flows themselves and in the induced ambient flow - changed abruptly with changes at the source. On the basis of my findings for unsteady laboratory jets, I conclude that variable eruption rates with characteristic time scales close to eruption duration have first-order control over volcanic plume evolution. Prior to my study, the significance of this variation was largely uncharacterized as the volcanology community predominately uses steady eruption models for interpretation and prediction of activity. My results suggest that unsteady models are necessary to accurately interpret behavior and assess threats from unsteady, short-lived eruptions.
ContributorsChojnicki, Kirsten (Author) / Clarke, Amanda (Thesis advisor) / Williams, Stanley (Committee member) / Adrian, Ronald (Committee member) / Phillips, Jeremy (Committee member) / Fernando, Harindra (Committee member) / Arizona State University (Publisher)
Created2012