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The nucleon resonance spectrum consists of many overlapping excitations. Polarization observables are an important tool for understanding and clarifying these spectra. While there is a large data base of differential cross sections for the process, very few data exist for polarization observables. A program of double polarization experiments has been conducted at Jefferson Lab using a tagged polarized photon beam and a frozen spin polarized target (FROST). The results presented here were taken during the first running period of FROST using the CLAS detector at Jefferson Lab with photon energies ranging from 329 MeV to 2.35 GeV. Data are presented for the E polarization observable for eta meson photoproduction on the proton from threshold (W=1500 MeV) to W=1900 MeV. Comparisons to the partial wave analyses of SAID and Bonn-Gatchina along with the isobar analysis of eta-MAID are made. These results will help distinguish between current theoretical predictions and refine future theories.
ContributorsMorrison, Brian (Author) / Ritchie, Barry (Thesis advisor) / Dugger, Michael (Committee member) / Shovkovy, Igor (Committee member) / Davies, Paul (Committee member) / Alarcon, Ricardo (Committee member) / Arizona State University (Publisher)
Created2011
Description
Mechanisms for oxygen reduction are proposed for three distinct cases covering two ionic liquids of fundamentally different archetypes and almost thirty orders of magnitude of proton activity. Proton activity is treated both extrinsically by varying the concentration and intrinsically by selecting proton donors with a wide range of aqueous pKa values. The mechanism of oxygen reduction in ionic liquids is introduced by way of the protic ionic liquid (pIL) triethylammonium triflate (TEATf) which shares some similarities with aqueous acid solutions. Oxygen reduction in TEATf begins as the one electron rate limited step to form superoxide, O2*-, which is then rapidly protonated by the pIL cation forming the perhydroxyl radical, HO2*. The perhydroxyl radical is further reduced to peroxidate (HO2-) and hydrogen peroxide in proportions in accordance with their pKa. The reaction does not proceed beyond this point due to the adsorption of the conjugate base triethylammine interfering with the disproportionation of hydrogen peroxide. This work demonstrates that this mechanism is consistent across Pt, Au, Pd, and Ag electrodes. Two related sets of experiments were performed in the inherently aprotic ionic liquid 1-butyl-2,3-dimethylimidazolium triflate (C4dMImTf). The first involved the titration of acidic species of varying aqueous pKa into the IL while monitoring the extent of oxygen reduction as a function of pKa and potential on Pt and glassy carbon (GC) electrodes. These experiments confirmed the greater propensity of Pt to reduce oxygen by its immediate and abrupt transition from one electron reduction to four electron reduction, while oxygen reduction on GC gradually approaches four electron reduction as the potentials were driven more cathodic. The potential at which oxygen reduction initiates shows general agreement with the Nernst equation and the acid's tabulated aqueous pKa value, however at the extremely acidic end, a small deviation is observed. The second set of experiments in C4dMImTf solicited water as the proton donor for oxygen reduction in an approximation of the aqueous alkaline case. The water content was varied between extremely dry (<0.1 mol% H2O) and saturated (approximately 15.8 mol% H2O}). As the water content increased so too did the extent of oxygen reduction eventually approach two electrons on both Pt and GC. However, additional water led to a linear increase in the Tafel slope under enhanced mass transport conditions up to the point of 10 mol% water. This inhibition of oxygen adsorption is the result of the interaction between superoxide and water and more specifically is proposed to be associated with decomposition of theC4dMIm+ cation by hydroxide at the elevated temperatures required for the experiment. Oxygen reduction on both Pt and GC follows Nernstian behavior as the water content is increased. Separate mechanisms for oxygen reduction on Pt and GC are proposed based on the nature of the Nernstian response in these systems.
ContributorsZeller, Robert August (Author) / Friesen, Cody (Thesis advisor) / Sieradzki, Karl (Committee member) / Buttry, Daniel (Committee member) / Arizona State University (Publisher)
Created2011
Description
Preliminary feasibility studies for two possible experiments with the GlueX detector, installed in Hall D of Jefferson Laboratory, are presented. First, a general study of the feasibility of detecting the ηC at the current hadronic rate is discussed, without regard for detector or reconstruction efficiency. Second, a study of the use of statistical methods in studying exotic meson candidates is outlined, describing methods and providing preliminary data on their efficacy.
ContributorsPrather, Benjamin Scott (Author) / Ritchie, Barry G. (Thesis director) / Dugger, Michael (Committee member) / Barrett, The Honors College (Contributor) / School of Mathematical and Statistical Sciences (Contributor) / Department of Physics (Contributor)
Created2015-05
Description
A search is underway to find baryon resonances that have been predicted, but yet remain unobserved. Nucleon resonances, due to their broad energy widths, overlap and must be disentangled in order to be identified. Meson photoproduction observables related to the orientation of the spin of the incoming photon and the spin of the target proton are useful tools to deconvolve the nucleon resonance spectrum. These observables are particularly sensitive to interference between phases of the complex amplitudes. A set of these observables has been measured using the CEBAF Large Acceptance Spectrometer (CLAS) at Jefferson Lab with linearly-polarized photons having energies from 725 to 1575 MeV with polar angle values of cos(theta) between -0.8 and 0.9 and transversely-polarized protons in the Jefferson Lab FRozen Spin Target (FROST). By fitting neutron yields from gamma p -> pi^+ n over azimuthal scattering angle, the observables \H and P have been extracted. These observables manifest as azimuthal modulations in the yields for the double-polarization experiment. Preliminary results for these observables will be presented and compared with predictions provided by the SAID Partial-Wave Analysis Facility.
ContributorsLee, Robert John (Author) / Dugger, Michael (Thesis director) / Ritchie, Barry (Committee member) / Department of Physics (Contributor) / Barrett, The Honors College (Contributor)
Created2018-05
Description
The field of Ionic Liquid (IL) research has received considerable attention during the past decade. Unique physicochemical properties of these low melting salts have made them very promising for applications in a many areas of science and technology such as electrolyte research, green chemistry and electrodeposition. One of the most important parameters dictating their physicochemical behavior is the basicity of their anion. Using four sets of Protic Ionic Liquids (PILs) and spectroscopic characterization of them, a qualitative order for anion basicity of ILs is obtained.
Protic Ionic Liquids are made by proton transfer form a Brønsted acid to a base. The extent of this transfer is determined by the free energy change of the proton transfer process. For the cases with large enough free energy change during the process, the result is a fully ionic material whereas if the proton transfer is not complete, a mixture of ions, neutral molecules and aggregates is resulted. NMR and IR spectroscopies along with electrochemical and mechanical characterization of four sets of PILs are used to study the degree of ionicity.
Protic Ionic Liquids are made by proton transfer form a Brønsted acid to a base. The extent of this transfer is determined by the free energy change of the proton transfer process. For the cases with large enough free energy change during the process, the result is a fully ionic material whereas if the proton transfer is not complete, a mixture of ions, neutral molecules and aggregates is resulted. NMR and IR spectroscopies along with electrochemical and mechanical characterization of four sets of PILs are used to study the degree of ionicity.
ContributorsHasani, Mohammad (Author) / Angell, C. Austen (Thesis advisor) / Yarger, Jeffrey L (Committee member) / Gould, Ian R (Committee member) / Arizona State University (Publisher)
Created2016
Description
A series of experiments using a polarized beam incident on a polarized frozen spin target
(FROST) was conducted at Jefferson Lab in 2010. Results presented here were taken
during the second running period with the FROST target using the CEBAF Large Acceptance
Spectrometer (CLAS) detector at Jefferson Lab, which used transversely-polarized
protons in a butanol target and a circularly-polarized incident tagged photon beam with
energies between 0.62 and 2.93 GeV. Data are presented for the F and T polarization observables
for h meson photoproduction on the proton from W = 1.55 GeV to 1.80 GeV.
The data presented here will improve the world database and refine theoretical approaches
of nucleon structure.
(FROST) was conducted at Jefferson Lab in 2010. Results presented here were taken
during the second running period with the FROST target using the CEBAF Large Acceptance
Spectrometer (CLAS) detector at Jefferson Lab, which used transversely-polarized
protons in a butanol target and a circularly-polarized incident tagged photon beam with
energies between 0.62 and 2.93 GeV. Data are presented for the F and T polarization observables
for h meson photoproduction on the proton from W = 1.55 GeV to 1.80 GeV.
The data presented here will improve the world database and refine theoretical approaches
of nucleon structure.
ContributorsTucker, Ross (Author) / Ritchie, Barry (Thesis advisor) / Dugger, Michael (Committee member) / Alarcon, Ricardo (Committee member) / Lebed, Richard (Committee member) / Arizona State University (Publisher)
Created2016
Description
The OLYMPUS experiment measured the two-photon exchange contribution to elastic electron-proton scattering, over a range of four-momentum transfer from \(0.6 < Q^2 < 2.2\) \((\mathrm{GeV/c})^2\). The motivation for the experiment stemmed from measurements of the electric-to-magnetic form factor ratio of the proton \(\mu G_E/G_M\) extracted from polarization observables in polarized electron-proton scattering. Polarized electron-proton scattering experiments have revealed a significant decrease in \(\mu G_E/G_M\) at large \(Q^2\), in contrast to previous measurements from unpolarized electron-proton scattering. The commonly accepted hypothesis is that the discrepancy in the form factor ratio is due to neglected higher-order terms in the elastic electron-proton scattering cross section, in particular the two-photon exchange amplitude.
The goal of OLYMPUS was to measure the two-photon exchange contribution by measuring the positron-proton to electron-proton elastic scattering cross section ratio, \(\sigma_{e^+p}/\sigma_{e^-p}\). The two-photon exchange contribution is correlated to the deviation of the cross section ratio from unity.
In 2012, the OLYMPUS experiment collected over 4 fb\(^{-1}\) of \(e^+p\) and \(e^-p\) scattering data using electron and positron beams incident on a hydrogen gas target. The scattered leptons and protons were measured exclusively with a large acceptance spectrometer. OLYMPUS observed a slight rise in \(\sigma_{e^+p}/\sigma_{e^-p}\) of at most 1-2\% over a \(Q^2\) range of \(0.6 < Q^2 < 2.2\) \((\mathrm{GeV/c})^2\). This work discusses the motivations, experiment, analysis method, and the preliminary results for the cross section ratio as measured by OLYMPUS.
The goal of OLYMPUS was to measure the two-photon exchange contribution by measuring the positron-proton to electron-proton elastic scattering cross section ratio, \(\sigma_{e^+p}/\sigma_{e^-p}\). The two-photon exchange contribution is correlated to the deviation of the cross section ratio from unity.
In 2012, the OLYMPUS experiment collected over 4 fb\(^{-1}\) of \(e^+p\) and \(e^-p\) scattering data using electron and positron beams incident on a hydrogen gas target. The scattered leptons and protons were measured exclusively with a large acceptance spectrometer. OLYMPUS observed a slight rise in \(\sigma_{e^+p}/\sigma_{e^-p}\) of at most 1-2\% over a \(Q^2\) range of \(0.6 < Q^2 < 2.2\) \((\mathrm{GeV/c})^2\). This work discusses the motivations, experiment, analysis method, and the preliminary results for the cross section ratio as measured by OLYMPUS.
ContributorsIce, Lauren (Author) / Alarcon, Ricardo O (Thesis advisor) / Dugger, Michael (Committee member) / Lebed, Richard (Committee member) / Ritchie, Barry (Committee member) / Arizona State University (Publisher)
Created2016
Description
The GlueX experiment housed in Hall D of the Thomas Jefferson National Laboratory was created to map the light meson spectrum in order to contribute to the Standard Model of particle physics by strengthening our understanding of the strong interaction. GlueX is a medium-energy photoproduction experiment that utilizes a linearly polarized photon beam to create hadronic forms of matter. By mapping the light meson spectrum, the GlueX collaboration hopes to identify meson states forbidden by the Constituent Quark Model. As a main research objective, the GlueX collaboration is searching for hybrid $q\bar{q}g$ meson states that exhibit exotic quantum numbers. One hybrid meson candidate is the $\eta'_1$, which is predicted to decay to $K^\ast\bar{K}$ and have a mass near $2.3~\mathrm{GeV}$ (\citeauthor{qn_exotic_status}, \citeyear{qn_exotic_status}; \citeauthor{hybrid_mesons}, \citeyear{hybrid_mesons}). At this time, very few meson states have been identified in the $2.0~\mathrm{GeV}$ mass region. This dearth of evidence for existing states requires any tool developed to search for meson states above $2.0~\mathrm{GeV}$ must be verified by looking at known meson states. In order to search for the $\eta'_1$ hybrid meson candidate in $\gamma p \rightarrow pK^+K^-\gamma\gamma$ events, meson states decaying $K^\ast\bar{K}$ that contribute to the low mass region must be identified, defined in this document as particles having masses between $1400$ and $1600~\mathrm{MeV}$. Identifying what meson states exist in the low mass region is also critical to mapping the light meson spectrum and determining the quark-gluonic content of those meson states. The results of a partial wave analysis (PWA) of $\gamma p \rightarrow pX$ where $X\rightarrow K^\ast\bar{K}$ from $\gamma p \rightarrow pK^+K^-\gamma\gamma$ events in GlueX are presented. In the $J=0$ invariant mass distribution, the $\eta(1405)$ and $\eta(1475)$ are identified, adding to the debate as to whether two pseudoscalar mesons exist in the low mass region. For the $J=1$ distribution, the $f_1(1420)$ and $f_1(1510)$ axial vector mesons are seen, where the former helps further elaborate on the $E\iota$ puzzle of the twentieth century \citep{E_iota_puzzle}. With respect to the controversy of meson states in the low mass region, evidence for the existence of the $f_2(1430)$ meson is strengthened in the $J=2$ distribution, and the $f'_2(1525)$ state is seen. This work lays a foundation for the ASU Meson Physics Group to continue a wider search for hybrid mesons in the $\gamma p \rightarrow pK^+K^-\gamma\gamma$ reaction topology.
ContributorsCole, Sebastian Miles (Author) / Dugger, Michael (Thesis advisor) / Ritchie, Barry (Committee member) / Alarcon, Ricardo (Committee member) / Shovkovy, Igor (Committee member) / Arizona State University (Publisher)
Created2021