Matching Items (3)
Filtering by

Clear all filters

170566-Thumbnail Image.png
Description

Workshop report on socio-economic and technical discussions Direct Air Capture as a technology for the climate transition.

Created2022-01-19
171967-Thumbnail Image.png
Description
Climate change poses a serious challenge humankind. Society’s reliance on fossil fuels raises atmospheric CO2 concentrations causing global warming. Already, the planet has warmed by 1.1 °C making it nearly impossible to heed the advice of the IPCC (2022) and prevent warming in excess of 1.5 °C by 2050. Even

Climate change poses a serious challenge humankind. Society’s reliance on fossil fuels raises atmospheric CO2 concentrations causing global warming. Already, the planet has warmed by 1.1 °C making it nearly impossible to heed the advice of the IPCC (2022) and prevent warming in excess of 1.5 °C by 2050. Even the current excess of CO2 in the atmosphere poses significant risks. Direct air capture (DAC) of CO2 offers one of the most scalable options to the drawdown of carbon. DAC can collect CO2 that is already diluted into the atmosphere for disposal or utilization. Central to most DAC are sorbents, i.e., materials that bind and release CO2 in a capture and release cycle. There are sorbents that cycle through a temperature swing. Others use a moisture swing, or a pressure swing or combinations of all of them. Since DAC is still a nascent technology, advancement of sorbents is an important part of DAC development. There is a nearly infinite combination of possible sorbents and form factors of sorbents that can be deployed in many different variations of DAC. Our goal is to develop a methodology for characterizing sorbents to facilitate rational choices among different options. Good sorbent characteristics include high capacity, fast sorption and desorption kinetics, low energy need for unloading, and longevity. This work presents the development of a systematic approach to evaluate sorbents from the milligram to tonne scale focusing on the important characteristics mentioned above. The work identified a good temperature swing sorbent whose characterization moved from the mg to kg scale without loss in performance. This work represents a first step in systematizing sorbent characterization for rational sorbent development programs.
ContributorsStangherlin Barbosa, Thiago (Author) / Lackner, Klaus (Thesis advisor) / Cirucci, John (Committee member) / Dirks, Gary (Committee member) / Arizona State University (Publisher)
Created2022
154691-Thumbnail Image.png
Description
This thesis examines the use of the moisture swing resin materials employed at the Center for Negative Carbon Emissions (CNCE) in order to provide carbon dioxide from ambient air to photobioreactors containing extremophile cyanobacteria cultured at the Arizona Center for Algae Technology and Innovation (AzCATI). For this purpose, a

This thesis examines the use of the moisture swing resin materials employed at the Center for Negative Carbon Emissions (CNCE) in order to provide carbon dioxide from ambient air to photobioreactors containing extremophile cyanobacteria cultured at the Arizona Center for Algae Technology and Innovation (AzCATI). For this purpose, a carbon dioxide feeding device was designed, built, and tested. The results indicate how much resin should be used with a given volume of algae medium: approximately 500 grams of resin can feed 1% CO2 at about three liters per minute to a ten liter medium of the Galdieria sulphuraria 5587.1 strain for one hour (equivalent to about 0.1 grams of carbon dioxide per hour per seven grams of algae). Using the resin device, the algae grew within their normal growth range: 0.096 grams of ash-free dry weight per liter over a six hour period. Future applications in which the resin-to-algae process can be utilized are discussed.
ContributorsBeaubien, Courtney (Author) / Lackner, Klaus (Thesis advisor) / Lammers, Peter (Committee member) / Atkins, Steve (Committee member) / Arizona State University (Publisher)
Created2016