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This dissertation presents research findings regarding the exploitation of localized surface plasmon (LSP) of epitaxial Ag islands as a means to enhance the photoluminescence (PL) of Germanium (Ge) quantum dots (QDs). The first step of this project was to investigate the growth of Ag islands on Si(100). Two distinct families

This dissertation presents research findings regarding the exploitation of localized surface plasmon (LSP) of epitaxial Ag islands as a means to enhance the photoluminescence (PL) of Germanium (Ge) quantum dots (QDs). The first step of this project was to investigate the growth of Ag islands on Si(100). Two distinct families of Ag islands have been observed. “Big islands” are clearly faceted and have basal dimensions in the few hundred nm to μm range with a variety of basal shapes. “Small islands” are not clearly faceted and have basal diameters in the 10s of nm range. Big islands form via a nucleation and growth mechanism, and small islands form via precipitation of Ag contained in a planar layer between the big islands that is thicker than the Stranski-Krastanov layer existing at room-temperature.

The pseudodielectric functions of epitaxial Ag islands on Si(100) substrates were investigated with spectroscopic ellipsometry. Comparing the experimental pseudodielectric functions obtained for Si with and without Ag islands clearly identifies a plasmon mode with its dipole moment perpendicular to the surface. This observation is confirmed using a simulation based on the thin island film (TIF) theory. Another mode parallel to the surface may be identified by comparing the experimental pseudodielectric functions with the simulated ones from TIF theory. Additional results suggest that the LSP energy of Ag islands can be tuned from the ultra-violet to the infrared range by an amorphous Si (α-Si) cap layer.

Heterostructures were grown that incorporated Ge QDs, an epitaxial Si cap layer and Ag islands grown atop the Si cap layer. Optimum growth conditions for distinct Ge dot ensembles and Si cap layers were obtained. The density of Ag islands grown on the Si cap layer depends on its thickness. Factors contributing to this effect may include the average strain and Ge concentration on the surface of the Si cap layer.

The effects of the Ag LSP on the PL of Ge coherent domes were investigated for both α-Si capped and bare Ag islands. For samples with low-doped substrates, the LSPs reduce the Ge dot-related PL when the Si cap layer is below some critical thickness and have no effect on the PL when the Si cap layer is above the critical thickness. For samples grown on highly-doped wafers, the LSP of bare Ag islands enhanced the PL of Ge QDs by ~ 40%.
ContributorsKong, Dexin (Author) / Drucker, Jeffery (Thesis advisor) / Chen, Tingyong (Committee member) / Ros, Robert (Committee member) / Smith, David (Committee member) / Arizona State University (Publisher)
Created2015
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In this experiment, an attempt was made to measure the index of refraction of a thin glass microscope slide, with a known thickness of 1.01 mm. A monochromatic laser with wavelength of 532nm was employed to generate the interference pattern through the use of a Michelson interferometer. The slide was

In this experiment, an attempt was made to measure the index of refraction of a thin glass microscope slide, with a known thickness of 1.01 mm. A monochromatic laser with wavelength of 532nm was employed to generate the interference pattern through the use of a Michelson interferometer. The slide was placed in the path of one of the beams. The slide could then be rotated through a series of angles, and, from the resulting changes in the interference pattern, the index of refraction of the slide could be extracted. The index of refraction was found to be 1.5±0.02.
ContributorsSwenson, Jordan (Author) / Sukharev, Maxim (Thesis director) / Bennett, Peter (Committee member) / Barrett, The Honors College (Contributor) / Department of Physics (Contributor)
Created2014-05
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Within the context of the Finite-Difference Time-Domain (FDTD) method of simulating interactions between electromagnetic waves and matter, we adapt a known absorbing boundary condition, the Convolutional Perfectly-Matched Layer (CPML) to a background of Drude-dispersive medium. The purpose of this CPML is to terminate the virtual grid of scattering simulations by

Within the context of the Finite-Difference Time-Domain (FDTD) method of simulating interactions between electromagnetic waves and matter, we adapt a known absorbing boundary condition, the Convolutional Perfectly-Matched Layer (CPML) to a background of Drude-dispersive medium. The purpose of this CPML is to terminate the virtual grid of scattering simulations by absorbing all outgoing radiation. In this thesis, we exposit the method of simulation, establish the Perfectly-Matched Layer as a domain which houses a spatial-coordinate transform to the complex plane, construct the CPML in vacuum, adapt the CPML to the Drude medium, and conclude with tests of the adapted CPML for two different scattering geometries.
ContributorsThornton, Brandon Maverick (Author) / Sukharev, Maxim (Thesis director) / Goodnick, Stephen (Committee member) / School of Mathematical and Statistical Sciences (Contributor) / Department of Physics (Contributor) / Barrett, The Honors College (Contributor)
Created2018-05
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Description

As the search for life in our universe grows, it is important to not only locate planets outside of our solar system, but also to work towards the ability to understand and characterize their nature. Many current research endeavors focus on the discovery of exoplanets throughout the surrounding universe; however,

As the search for life in our universe grows, it is important to not only locate planets outside of our solar system, but also to work towards the ability to understand and characterize their nature. Many current research endeavors focus on the discovery of exoplanets throughout the surrounding universe; however, we still know very little about the characteristics of these exoplanets themselves, particularly their atmospheres. Observatories, such as the Hubble Space Telescope and the Spitzer Space Telescope, have made some of the first observations which revealed information about the atmospheres of exoplanets but have yet to acquire complete and detailed characterizations of exoplanet atmospheres. The EXoplanet Climate Infrared TElescope (EXCITE) is a mission specifically designed to target key information about the atmospheres of exoplanets - including the global and spatially resolved energy budget, chemical bulk-compositions, vertical temperature profiles and circulation patterns across the surface, energy distribution efficiency as a function of equilibrium temperatures, and cloud formation and distribution - in order to generate dynamic and detailed atmospheric characterizations. EXCITE will use phase-resolved transit spectroscopy in the 1-4 micron wavelength range to accomplish these science goals, so it is important that the EXCITE spectrograph system is designed and tested to meet these observational requirements. For my thesis, I present my research on the EXCITE mission science goals and the design of the EXCITE spectrograph system to meet these goals, along with the work I have done in the beginning stages of testing the EXCITE spectrograph system in the lab. The primary result of my research work is the preparation of a simple optics setup in the lab to prepare a laser light source for use in the EXCITE spectrograph system - comparable to the preparation of incoming light by the EXCITE telescope system - which successfully yields an F# = 12.9 and a spot size of s = 39 ± 7 microns. These results meet the expectations of the system and convey appropriate preparation of a light source to begin the assembly and testing of the EXCITE spectrograph optics in the lab.

ContributorsHorvath, Zoe (Author) / Butler, Nathaniel (Thesis director) / Line, Michael (Committee member) / Scowen, Paul (Committee member) / Barrett, The Honors College (Contributor) / School of Earth and Space Exploration (Contributor) / Department of Physics (Contributor)
Created2022-05